J. A. Budagosky, D. V. Khomitsky, E. Ya. Sherman, and A. Castro, Phys. Rev. B 93, 035423 (2016).

We use quantum optimal control theory algorithms to design external electric fields that drive the coupled spin and orbital dynamics of an electron in a double quantum dot, subject to the spin-orbit coupling and Zeeman magnetic fields. We obtain time profiles of multifrequency electric field pulses which increase the rate of spin-flip transitions by several orders of magnitude in comparison with monochromatic fields, where the spin Rabi oscillations were predicted to be very slow. This precise (with fidelity higher than 1 × 10−4 ) and fast (at the time scale of the order of 0.1 ns, comparable with the Zeeman spin rotation and the interdot tunneling time) simultaneous control of the spin and position is achieved while keeping the electron in the four lowest tunneling and Zeeman-split levels through the duration of the pulse. The proposed algorithms suggest effective applications in spintronics and quantum information devices.